Computational studies on linear and third-order nonlinear optical phenomena of dipolar subunits described for an octupolar system

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Tarih

2019

Dergi Başlığı

Dergi ISSN

Cilt Başlığı

Yayıncı

IEEE Computer Society

Erişim Hakkı

info:eu-repo/semantics/closedAccess

Özet

We have computed the electric dipole moments (μ), dispersion-free and frequency-dependent dipole polarizabilities (α) and third-order hyperpolarizabilities (γ) of dipolar subunits described for an octupolar system (1-3) utilizing time-dependent Hartree-Fock (TDHF) approach. To conceive the nonlinear optical (NLO) phenomena, the third-order susceptibilities (χ(3)) for the title structures have been also derived from the abinitio quantum mechanical procedure (TDHF). According to the computed data on the NLO properties; the cubic hyperpolarizability and susceptibility results of 1-3 are considerably coherent with the measurement values initially produced. © 2019 IEEE.

Açıklama

APEX Technologies; CNRS; HV Photonics; Lumomat; Moltech Anjou; Springer
21st International Conference on Transparent Optical Networks, ICTON 2019 -- 9 July 2019 through 13 July 2019 -- Angers -- 152064

Anahtar Kelimeler

Second hyperpolarizability, Third-order optical nonlinearity, Third-order susceptibility, Time-dependent Hartree-Fock

Kaynak

International Conference on Transparent Optical Networks

WoS Q Değeri

Scopus Q Değeri

N/A

Cilt

2019-July

Sayı

Künye